01739nas a2200205 4500008004100000245013400041210006900175260001500244520106400259100001801323700001201341700002201353700001701375700002501392700001301417700001901430700002601449700002101475856003701496 2019 eng d00aFeshbach resonances in p-wave three-body recombination within Fermi-Fermi mixtures of open-shell 6Li and closed-shell 173Yb atoms0 aFeshbach resonances in pwave threebody recombination within Ferm c12/10/20193 a

We report on observations and modeling of interspecies magnetic Feshbach resonances in dilute ultracold mixtures of open-shell alkali-metal 6Li and closed-shell 173Yb atoms with temperatures just above quantum degeneracy for both fermionic species. Resonances are located by detecting magnetic-field-dependent atom loss due to three-body recombination. We resolve closely-located resonances that originate from a weak separation-dependent hyperfine coupling between the electronic spin of 6Li and the nuclear spin of 173Yb, and confirm their magnetic field spacing by ab initio electronic-structure calculations. Through quantitative comparisons of theoretical atom-loss profiles and experimental data at various temperatures between 1 μK and 20 μK, we show that three-body recombination in fermionic mixtures has a p-wave Wigner threshold behavior leading to characteristic asymmetric loss profiles. Such resonances can be applied towards the formation of ultracold doublet ground-state molecules and quantum simulation of superfluid p-wave pairing.

1 aGreen, Alaina1 aLi, Hui1 aToh, Jun, Hui See1 aTang, Xinxin1 aMcCormick, Katherine1 aLi, Ming1 aTiesinga, Eite1 aKotochigova, Svetlana1 aGupta, Subhadeep uhttps://arxiv.org/abs/1912.0487401691nas a2200169 4500008004100000245007000041210006900111260001500180300001300195490000600208520118500214100002701399700001301426700001901439700002601458856003701484 2018 eng d00aFractal Universality in Near-Threshold Magnetic Lanthanide Dimers0 aFractal Universality in NearThreshold Magnetic Lanthanide Dimers c2018/02/16 aeaap83080 v43 a

Ergodic quantum systems are often quite alike, whereas nonergodic, fractal systems are unique and display characteristic properties. We explore one of these fractal systems, weakly bound dysprosium lanthanide molecules, in an external magnetic field. As recently shown, colliding ultracold magnetic dysprosium atoms display a soft chaotic behavior with a small degree of disorder. We broaden this classification by investigating the generalized inverse participation ratio and fractal dimensions for large sets of molecular wave functions. Our exact close-coupling simulations reveal a dynamic phase transition from partially localized states to totally delocalized states and universality in its distribution by increasing the magnetic field strength to only a hundred Gauss (or 10 mT). Finally, we prove the existence of nonergodic delocalized phase in the system and explain the violation of ergodicity by strong coupling between near-threshold molecular states and the nearby continuum.

1 aMakrides, Constantinos1 aLi, Ming1 aTiesinga, Eite1 aKotochigova, Svetlana uhttps://arxiv.org/abs/1802.0958601661nas a2200121 4500008004100000245009700041210006900138520123700207100001301444700001901457700002601476856003701502 2018 eng d00aOrbital quantum magnetism in spin dynamics of strongly interacting magnetic lanthanide atoms0 aOrbital quantum magnetism in spin dynamics of strongly interacti3 a

Laser cooled lanthanide atoms are ideal candidates with which to study strong and unconventional quantum magnetism with exotic phases. Here, we use state-of-the-art closed-coupling simulations to model quantum magnetism for pairs of ultracold spin-6 erbium lanthanide atoms placed in a deep optical lattice. In contrast to the widely used single-channel Hubbard model description of atoms and molecules in an optical lattice, we focus on the single-site multi-channel spin evolution due to spin-dependent contact, anisotropic van der Waals, and dipolar forces. This has allowed us to identify the leading mechanism, orbital anisotropy, that governs molecular spin dynamics among erbium atoms. The large magnetic moment and combined orbital angular momentum of the 4f-shell electrons are responsible for these strong anisotropic interactions and unconventional quantum magnetism. Multi-channel simulations of magnetic Cr atoms under similar trapping conditions show that their spin-evolution is controlled by spin-dependent contact interactions that are distinct in nature from the orbital anisotropy in Er. The role of an external magnetic field and the aspect ratio of the lattice site on spin dynamics is also investigated.

1 aLi, Ming1 aTiesinga, Eite1 aKotochigova, Svetlana uhttps://arxiv.org/abs/1804.1010201318nas a2200145 4500008004100000245008900041210006900130260001300199490000800212520084800220100002201068700001901090700002601109856003701135 2012 eng d00aAnisotropy induced Feshbach resonances in a quantum dipolar gas of magnetic atoms 0 aAnisotropy induced Feshbach resonances in a quantum dipolar gas  c2012/9/70 v1093 a We explore the anisotropic nature of Feshbach resonances in the collision between ultracold magnetic submerged-shell dysprosium atoms, which can only occur due to couplings to rotating bound states. This is in contrast to well-studied alkali-metal atom collisions, where most Feshbach resonances are hyperfine induced and due to rotation-less bound states. Our novel first-principle coupled-channel calculation of the collisions between open-4f-shell spin-polarized bosonic dysprosium reveals a striking correlation between the anisotropy due to magnetic dipole-dipole and electrostatic interactions and the Feshbach spectrum as a function of an external magnetic field. Over a 20 mT magnetic field range we predict about a dozen Feshbach resonances and show that the resonance locations are exquisitely sensitive to the dysprosium isotope. 1 aPetrov, Alexander1 aTiesinga, Eite1 aKotochigova, Svetlana uhttp://arxiv.org/abs/1203.4172v101547nas a2200157 4500008004100000245009000041210006900131260001500200300001100215490000700226520105100233100002601284700001901310700002301329856003701352 2009 eng d00aMulti-channel modelling of the formation of vibrationally cold polar KRb molecules 0 aMultichannel modelling of the formation of vibrationally cold po c2009/05/14 a0550430 v113 a We describe the theoretical advances that influenced the experimental creation of vibrationally and translationally cold polar $^{40}$K$^{87}$Rb molecules \cite{nphys08,science08}. Cold molecules were created from very-weakly bound molecules formed by magnetic field sweeps near a Feshbach resonance in collisions of ultra-cold $^{40}$K and $^{87}$Rb atoms. Our analysis include the multi-channel bound-state calculations of the hyperfine and Zeeman mixed X$^1\Sigma^+$ and a$^3\Sigma^+$ vibrational levels. We find excellent agreement with the hyperfine structure observed in experimental data. In addition, we studied the spin-orbit mixing in the intermediate state of the Raman transition. This allowed us to investigate its effect on the vibrationally-averaged transition dipole moment to the lowest ro-vibrational level of the X$^1\Sigma^+$ state. Finally, we obtained an estimate of the polarizability of the initial and final ro-vibrational states of the Raman transition near frequencies relevant for optical trapping of the molecules. 1 aKotochigova, Svetlana1 aTiesinga, Eite1 aJulienne, Paul, S. uhttp://arxiv.org/abs/0901.1486v101322nas a2200169 4500008004100000245007000041210006900111260001400180490000700194520079400201100002300995700002301018700002601041700001901067700002301086856004301109 2003 eng d00aUltracold collision properties of metastable alkaline-earth atoms0 aUltracold collision properties of metastable alkalineearth atoms c2003/2/130 v903 a Ultra-cold collisions of spin-polarized 24Mg,40Ca, and 88Sr in the metastable 3P2 excited state are investigated. We calculate the long-range interaction potentials and estimate the scattering length and the collisional loss rate as a function of magnetic field. The estimates are based on molecular potentials between 3P2 alkaline-earth atoms obtained from ab initio atomic and molecular structure calculations. The scattering lengths show resonance behavior due to the appearance of a molecular bound state in a purely long-range interaction potential and are positive for magnetic fields below 50 mT. A loss-rate model shows that losses should be smallest near zero magnetic field and for fields slightly larger than the resonance field, where the scattering length is also positive. 1 aDerevianko, Andrei1 aPorsev, Sergey, G.1 aKotochigova, Svetlana1 aTiesinga, Eite1 aJulienne, Paul, S. uhttp://arxiv.org/abs/physics/0210076v1