01979nas a2200277 4500008004100000245007600041210006900117260001400186520117400200100001301374700001801387700002101405700002901426700001601455700002001471700001801491700001501509700002001524700002301544700001801567700002101585700001801606700002101624700001901645856003701664 2021 eng d00aChiral transport of hot carriers in graphene in the quantum Hall regime0 aChiral transport of hot carriers in graphene in the quantum Hall c10/3/20213 a
Photocurrent (PC) measurements can reveal the relaxation dynamics of photo-excited hot carriers beyond the linear response of conventional transport experiments, a regime important for carrier multiplication. In graphene subject to a magnetic field, PC measurements are able to probe the existence of Landau levels with different edge chiralities which is exclusive to relativistic electron systems. Here, we report the accurate measurement of PC in graphene in the quantum Hall regime. Prominent PC oscillations as a function of gate voltage on samples' edges are observed. These oscillation amplitudes form an envelope which depends on the strength of the magnetic field, as does the PCs' power dependence and their saturation behavior. We explain these experimental observations through a model using optical Bloch equations, incorporating relaxations through acoustic-, optical- phonons and Coulomb interactions. The simulated PC agrees with our experimental results, leading to a unified understanding of the chiral PC in graphene at various magnetic field strengths, and providing hints for the occurrence of a sizable carrier multiplication.
1 aCao, Bin1 aGrass, Tobias1 aGazzano, Olivier1 aPatel, Kishan, Ashokbhai1 aHu, Jiuning1 aMüller, Markus1 aHuber, Tobias1 aAnzi, Luca1 aWatanabe, Kenji1 aTaniguchi, Takashi1 aNewell, David1 aGullans, Michael1 aSordan, Roman1 aHafezi, Mohammad1 aSolomon, Glenn uhttps://arxiv.org/abs/2110.01079